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Electronic properties of ultra-thin YCrO 3 films

We report on the heteroepitaxial stabilization of YCrO 3 ultra-thin films on LSAT (001) substrate. Using a combination of resonant X-ray absorption spectroscopy (XAS) and atomic multiplet cluster calculation, the electronic structure of YCrO 3 thin film was investigated. Polarization dependent Cr L... Full description

Journal Title: Applied Physics Letters 18 June 2018, Vol.112(25)
Main Author: Pal, Banabir
Other Authors: Liu, Xiaoran , Wen, Fangdi , Kareev, Mikhail , N'Diaye, A. T. , Shafer, P. , Arenholz, E. , Chakhalian, Jak
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: ISSN: 0003-6951 ; E-ISSN: 1077-3118 ; DOI: 10.1063/1.5029977
Link: http://dx.doi.org/10.1063/1.5029977
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recordid: aip_complete10.1063/1.5029977
title: Electronic properties of ultra-thin YCrO 3 films
format: Article
creator:
  • Pal, Banabir
  • Liu, Xiaoran
  • Wen, Fangdi
  • Kareev, Mikhail
  • N'Diaye, A. T.
  • Shafer, P.
  • Arenholz, E.
  • Chakhalian, Jak
subjects:
  • Dielectrics, Ferroelectrics, And Multiferroics
ispartof: Applied Physics Letters, 18 June 2018, Vol.112(25)
description: We report on the heteroepitaxial stabilization of YCrO 3 ultra-thin films on LSAT (001) substrate. Using a combination of resonant X-ray absorption spectroscopy (XAS) and atomic multiplet cluster calculation, the electronic structure of YCrO 3 thin film was investigated. Polarization dependent Cr L 3,2 edge XAS measurements reveal the presence of x-ray linear dichroism spectrum uncharacteristic of a 3 d 3 electronic system in an octahedral crystal field. Atomic multiplet calculation demonstrates the critical importance of charge transfer energy, coulomb correlation strength, and hopping interaction in realizing this dichroism spectrum.
language: eng
source:
identifier: ISSN: 0003-6951 ; E-ISSN: 1077-3118 ; DOI: 10.1063/1.5029977
fulltext: fulltext
issn:
  • 0003-6951
  • 1077-3118
  • 00036951
  • 10773118
url: Link


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ispartofApplied Physics Letters, 18 June 2018, Vol.112(25)
subjectDielectrics, Ferroelectrics, And Multiferroics
descriptionWe report on the heteroepitaxial stabilization of YCrO 3 ultra-thin films on LSAT (001) substrate. Using a combination of resonant X-ray absorption spectroscopy (XAS) and atomic multiplet cluster calculation, the electronic structure of YCrO 3 thin film was investigated. Polarization dependent Cr L 3,2 edge XAS measurements reveal the presence of x-ray linear dichroism spectrum uncharacteristic of a 3 d 3 electronic system in an octahedral crystal field. Atomic multiplet calculation demonstrates the critical importance of charge transfer energy, coulomb correlation strength, and hopping interaction in realizing this dichroism spectrum.
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descriptionWe report on the heteroepitaxial stabilization of YCrO 3 ultra-thin films on LSAT (001) substrate. Using a combination of resonant X-ray absorption spectroscopy (XAS) and atomic multiplet cluster calculation, the electronic structure of YCrO 3 thin film was investigated. Polarization dependent Cr L 3,2 edge XAS measurements reveal the presence of x-ray linear dichroism spectrum uncharacteristic of a 3 d 3 electronic system in an octahedral crystal field. Atomic multiplet calculation demonstrates the critical importance of charge transfer energy, coulomb correlation strength, and hopping interaction in realizing this dichroism spectrum.
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abstractWe report on the heteroepitaxial stabilization of YCrO 3 ultra-thin films on LSAT (001) substrate. Using a combination of resonant X-ray absorption spectroscopy (XAS) and atomic multiplet cluster calculation, the electronic structure of YCrO 3 thin film was investigated. Polarization dependent Cr L 3,2 edge XAS measurements reveal the presence of x-ray linear dichroism spectrum uncharacteristic of a 3 d 3 electronic system in an octahedral crystal field. Atomic multiplet calculation demonstrates the critical importance of charge transfer energy, coulomb correlation strength, and hopping interaction in realizing this dichroism spectrum.
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