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Degradation of organic compounds in a fenton system based on chitosan/Fe0/Fe2O3 composites: a theoretical and experimental study

Chitosan is a polymer with interesting characteristics for use in catalysis, such as biocompatibility, high chemical reactivity and stability under various conditions. Seeking new applications, a new hybrid material was synthesized for use in the degradation of organic compound. A synthesis route pr... Full description

Journal Title: Journal of the Iranian Chemical Society 2/2016, Vol.13(2), pp.377-386
Main Author: Ferreira, Laís O.
Other Authors: Lemos, Ana C. C. , Nogueira, Francisco G. E. , Guimaraes, Iara R. , Guerreiro, Mario C. , Rocha, Marcus V. J. , Savedra, Ranylson M. L. , Hammer, Peter , Brito, Angela D. B. , Da Cunha, Elaine F. F. , Silva, Joaquim P. , Ramalho, Teodorico C.
Format: Electronic Article Electronic Article
Language: English
Subjects:
Dye
ID: ISSN: 1735-207X ; E-ISSN: 1735-2428 ; DOI: http://dx.doi.org/10.1007/s13738-015-0746-1
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recordid: crossref10.1007/s13738-015-0746-1
title: Degradation of organic compounds in a fenton system based on chitosan/Fe0/Fe2O3 composites: a theoretical and experimental study
format: Article
creator:
  • Ferreira, Laís O.
  • Lemos, Ana C. C.
  • Nogueira, Francisco G. E.
  • Guimaraes, Iara R.
  • Guerreiro, Mario C.
  • Rocha, Marcus V. J.
  • Savedra, Ranylson M. L.
  • Hammer, Peter
  • Brito, Angela D. B.
  • Da Cunha, Elaine F. F.
  • Silva, Joaquim P.
  • Ramalho, Teodorico C.
subjects:
  • Chitosan
  • Fenton process
  • Iron
  • Dye
ispartof: Journal of the Iranian Chemical Society, 2/2016, Vol.13(2), pp.377-386
description: Chitosan is a polymer with interesting characteristics for use in catalysis, such as biocompatibility, high chemical reactivity and stability under various conditions. Seeking new applications, a new hybrid material was synthesized for use in the degradation of organic compound. A synthesis route proposed led to the formation of a material in the form of film. The characterization data indicated the presence of hematite, as well as metallic iron. In addition, a theoretical model for interaction of iron with chitosan was proposed. Molecular dynamics simulations indicate that non-Coulomb interactions modulate the adsorption process between reactive red dye and chitosan. The catalytic behavior of these hybrid materials was investigated for the H 2 O 2 decomposition to O 2 and the degradation of reactive red dye. The hybrid material showed high degradation capacity, confirming this material as an efficient heterogeneous Fenton catalysts.
language: eng
source:
identifier: ISSN: 1735-207X ; E-ISSN: 1735-2428 ; DOI: http://dx.doi.org/10.1007/s13738-015-0746-1
fulltext: fulltext
issn:
  • 1735207X
  • 1735-207X
  • 17352428
  • 1735-2428
url: Link


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titleDegradation of organic compounds in a fenton system based on chitosan/Fe0/Fe2O3 composites: a theoretical and experimental study
creatorFerreira, Laís O. ; Lemos, Ana C. C. ; Nogueira, Francisco G. E. ; Guimaraes, Iara R. ; Guerreiro, Mario C. ; Rocha, Marcus V. J. ; Savedra, Ranylson M. L. ; Hammer, Peter ; Brito, Angela D. B. ; Da Cunha, Elaine F. F. ; Silva, Joaquim P. ; Ramalho, Teodorico C.
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descriptionChitosan is a polymer with interesting characteristics for use in catalysis, such as biocompatibility, high chemical reactivity and stability under various conditions. Seeking new applications, a new hybrid material was synthesized for use in the degradation of organic compound. A synthesis route proposed led to the formation of a material in the form of film. The characterization data indicated the presence of hematite, as well as metallic iron. In addition, a theoretical model for interaction of iron with chitosan was proposed. Molecular dynamics simulations indicate that non-Coulomb interactions modulate the adsorption process between reactive red dye and chitosan. The catalytic behavior of these hybrid materials was investigated for the H 2 O 2 decomposition to O 2 and the degradation of reactive red dye. The hybrid material showed high degradation capacity, confirming this material as an efficient heterogeneous Fenton catalysts.
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date2016-02