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Pretreatment as the crucial step for biogas reforming to hydrogen over Ni–Co bimetallic catalyst: Effect of CO2 pretreatment time

γ-Al O pellets supported Ni–Co bimetallic catalyst prepared by excessive impregnation was employed for biogas reforming to hydrogen. H and CO pretreatment of the catalyst was investigated under different conditions in order to enhance the performance of the catalyst. CO pretreatment was performed at... Full description

Journal Title: International Journal of Hydrogen Energy 23 September 2014, Vol.39(28), pp.16195-16201
Main Author: Zhao, Jian
Other Authors: Zhou, Wei , Ma, Jianxin
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: ISSN: 0360-3199 ; E-ISSN: 1879-3487 ; DOI: 10.1016/j.ijhydene.2014.01.084
Link: https://www.sciencedirect.com/science/article/pii/S0360319914001347
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recordid: elsevier_sdoi_10_1016_j_ijhydene_2014_01_084
title: Pretreatment as the crucial step for biogas reforming to hydrogen over Ni–Co bimetallic catalyst: Effect of CO2 pretreatment time
format: Article
creator:
  • Zhao, Jian
  • Zhou, Wei
  • Ma, Jianxin
subjects:
  • Biogas Reforming
  • Hydrogen Production
  • Pretreatment
  • Time
  • Nickel–Cobalt Catalyst
  • Engineering
ispartof: International Journal of Hydrogen Energy, 23 September 2014, Vol.39(28), pp.16195-16201
description: γ-Al O pellets supported Ni–Co bimetallic catalyst prepared by excessive impregnation was employed for biogas reforming to hydrogen. H and CO pretreatment of the catalyst was investigated under different conditions in order to enhance the performance of the catalyst. CO pretreatment was performed at 850 °C and 0.1 MPa under different times (0, 0.25, 0.5, 1, 2 and 6 h). The activity is significantly increased by the pretreatment and has a close relationship with CO pretreatment time. No initial activation period was detected for catalyst with CO pretreatment for more than 0.5 h. The final conversion of methane increased from 87 to 95% and carbon dioxide from 95 to 99%, respectively, with increasing the CO pretreatment time from 0 to 1 h. Further increasing the pretreatment time from 1 to 6 h, the catalyst activity has a slight...
language: eng
source:
identifier: ISSN: 0360-3199 ; E-ISSN: 1879-3487 ; DOI: 10.1016/j.ijhydene.2014.01.084
fulltext: no_fulltext
issn:
  • 0360-3199
  • 03603199
  • 1879-3487
  • 18793487
url: Link


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titlePretreatment as the crucial step for biogas reforming to hydrogen over Ni–Co bimetallic catalyst: Effect of CO2 pretreatment time
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subjectBiogas Reforming ; Hydrogen Production ; Pretreatment ; Time ; Nickel–Cobalt Catalyst ; Engineering
descriptionγ-Al O pellets supported Ni–Co bimetallic catalyst prepared by excessive impregnation was employed for biogas reforming to hydrogen. H and CO pretreatment of the catalyst was investigated under different conditions in order to enhance the performance of the catalyst. CO pretreatment was performed at 850 °C and 0.1 MPa under different times (0, 0.25, 0.5, 1, 2 and 6 h). The activity is significantly increased by the pretreatment and has a close relationship with CO pretreatment time. No initial activation period was detected for catalyst with CO pretreatment for more than 0.5 h. The final conversion of methane increased from 87 to 95% and carbon dioxide from 95 to 99%, respectively, with increasing the CO pretreatment time from 0 to 1 h. Further increasing the pretreatment time from 1 to 6 h, the catalyst activity has a slight...
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