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Ti–V–Mn based metal hydrides for hydrogen storage

Two Ti–V–Mn BCC-Laves phase alloys with the nominal composition Ti V Mn ( = −0.04 and 0.01), were synthesised by arc melting. This compositional difference resulted in different compositions and unit cell volumes for the C14 Laves phase. Ti V Mn and Ti V Mn demonstrated reversible hydrogen sorption... Full description

Journal Title: Journal of Alloys and Compounds 15 December 2013, Vol.580, pp.S233-S237
Main Author: Pickering, Lydia
Other Authors: Li, Jing , Reed, Daniel , Bevan, Alexander I , Book, David
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: ISSN: 0925-8388 ; E-ISSN: 1873-4669 ; DOI: 10.1016/j.jallcom.2013.03.208
Link: https://www.sciencedirect.com/science/article/pii/S0925838813007652
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recordid: elsevier_sdoi_10_1016_j_jallcom_2013_03_208
title: Ti–V–Mn based metal hydrides for hydrogen storage
format: Article
creator:
  • Pickering, Lydia
  • Li, Jing
  • Reed, Daniel
  • Bevan, Alexander I
  • Book, David
subjects:
  • Hydrogen Storage Materials
  • Ti–V Based Alloys
  • X-Ray Diffraction
  • Microstructure
  • Hydrogen Absorption–Desorption
  • Engineering
  • Chemistry
  • Physics
ispartof: Journal of Alloys and Compounds, 15 December 2013, Vol.580, pp.S233-S237
description: Two Ti–V–Mn BCC-Laves phase alloys with the nominal composition Ti V Mn ( = −0.04 and 0.01), were synthesised by arc melting. This compositional difference resulted in different compositions and unit cell volumes for the C14 Laves phase. Ti V Mn and Ti V Mn demonstrated reversible hydrogen sorption capacities of 1.53 and 1.56 ± 0.05 wt.% (at 120 bar H at 303 K) respectively, however, the change in composition results in a small change in the enthalpy of hydride decomposition, and a significant change in plateau pressure and hysteresis. This may allow for the plateau pressure to be tuned to meet the requirements of different solid-state hydrogen storage applications.
language: eng
source:
identifier: ISSN: 0925-8388 ; E-ISSN: 1873-4669 ; DOI: 10.1016/j.jallcom.2013.03.208
fulltext: fulltext
issn:
  • 0925-8388
  • 09258388
  • 1873-4669
  • 18734669
url: Link


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subjectHydrogen Storage Materials ; Ti–V Based Alloys ; X-Ray Diffraction ; Microstructure ; Hydrogen Absorption–Desorption ; Engineering ; Chemistry ; Physics
descriptionTwo Ti–V–Mn BCC-Laves phase alloys with the nominal composition Ti V Mn ( = −0.04 and 0.01), were synthesised by arc melting. This compositional difference resulted in different compositions and unit cell volumes for the C14 Laves phase. Ti V Mn and Ti V Mn demonstrated reversible hydrogen sorption capacities of 1.53 and 1.56 ± 0.05 wt.% (at 120 bar H at 303 K) respectively, however, the change in composition results in a small change in the enthalpy of hydride decomposition, and a significant change in plateau pressure and hysteresis. This may allow for the plateau pressure to be tuned to meet the requirements of different solid-state hydrogen storage applications.
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