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Structural and spectroscopic characterization of a monomeric side-on manganese(IV) peroxo complex

Gotcha: The binding and activation of oxygen by a manganese complex is reported. A PS sub(3) coordination sphere built around a manganese(I) center facilitates the isolation of a monomeric manganese(IV) peroxo complex that is stable at ambient temperature (see picture). The activation of molecular o... Full description

Journal Title: Angewandte Chemie (International ed. in English) 29 May 2012, Vol.51(22), pp.5427-30
Main Author: Lee, Chien-Ming
Other Authors: Chuo, Chi-He , Chen, Ching-Hui , Hu, Cho-Chun , Chiang, Ming-Hsi , Tseng, Yu-Jan , Hu, Ching-Han , Lee, Gene-Hsiang
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; PMID: 22511384 Version:1 ; DOI: 10.1002/anie.201201735
Link: http://pubmed.gov/22511384
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recordid: medline22511384
title: Structural and spectroscopic characterization of a monomeric side-on manganese(IV) peroxo complex
format: Article
creator:
  • Lee, Chien-Ming
  • Chuo, Chi-He
  • Chen, Ching-Hui
  • Hu, Cho-Chun
  • Chiang, Ming-Hsi
  • Tseng, Yu-Jan
  • Hu, Ching-Han
  • Lee, Gene-Hsiang
subjects:
  • Manganese -- Chemistry
  • Organometallic Compounds -- Chemistry
  • Oxygen -- Chemistry
ispartof: Angewandte Chemie (International ed. in English), 29 May 2012, Vol.51(22), pp.5427-30
description: Gotcha: The binding and activation of oxygen by a manganese complex is reported. A PS sub(3) coordination sphere built around a manganese(I) center facilitates the isolation of a monomeric manganese(IV) peroxo complex that is stable at ambient temperature (see picture). The activation of molecular oxygen is proposed via a manganese(II) intermediate with an empty site for the binding of the substrate.
language: eng
source:
identifier: E-ISSN: 1521-3773 ; PMID: 22511384 Version:1 ; DOI: 10.1002/anie.201201735
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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descriptionGotcha: The binding and activation of oxygen by a manganese complex is reported. A PS sub(3) coordination sphere built around a manganese(I) center facilitates the isolation of a monomeric manganese(IV) peroxo complex that is stable at ambient temperature (see picture). The activation of molecular oxygen is proposed via a manganese(II) intermediate with an empty site for the binding of the substrate.
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