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Zeolite-encapsulated Mn(II) complexes as catalysts for selective alkene oxidation

Encapsulation of cis-(Mn(bpy)2)27 complexes in the supercages of zeolites X and Y catalyzes the selective epoxidation of alkenes without intrusions from self-oxidation or catalase activity processes. Acid-catalyzed ring-opening, carbon-carbon bond cleavage and alkenedioic acid production accompany t... Full description

Journal Title: Nature 1994, Vol.369(6481), p.543
Main Author: Peter-Paul Knops-Gerrits
Other Authors: Dirk De Vos , Frédéric Thibault-Starzyk , Pierre A. Jacobs
Format: Electronic Article Electronic Article
Language:
Subjects:
ID: ISSN: 0028-0836 ; E-ISSN: 1476-4687 ; DOI: 10.1038/369543a0
Link: http://dx.doi.org/10.1038/369543a0
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recordid: nature_a10.1038/369543a0
title: Zeolite-encapsulated Mn(II) complexes as catalysts for selective alkene oxidation
format: Article
creator:
  • Peter-Paul Knops-Gerrits
  • Dirk De Vos
  • Frédéric Thibault-Starzyk
  • Pierre A. Jacobs
subjects:
  • Zeolites -- Research
  • Manganese (Metal) -- Research
ispartof: Nature, 1994, Vol.369(6481), p.543
description: Encapsulation of cis-(Mn(bpy)2)27 complexes in the supercages of zeolites X and Y catalyzes the selective epoxidation of alkenes without intrusions from self-oxidation or catalase activity processes. Acid-catalyzed ring-opening, carbon-carbon bond cleavage and alkenedioic acid production accompany the epoxidation of cycloalkenes. Inhibition of reaction conditions and zeolite acidity selectively derive the various intermediates in the process.
language:
source:
identifier: ISSN: 0028-0836 ; E-ISSN: 1476-4687 ; DOI: 10.1038/369543a0
fulltext: fulltext
issn:
  • 0028-0836
  • 00280836
  • 1476-4687
  • 14764687
url: Link


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titleZeolite-encapsulated Mn(II) complexes as catalysts for selective alkene oxidation
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descriptionEncapsulation of cis-(Mn(bpy)2)27 complexes in the supercages of zeolites X and Y catalyzes the selective epoxidation of alkenes without intrusions from self-oxidation or catalase activity processes. Acid-catalyzed ring-opening, carbon-carbon bond cleavage and alkenedioic acid production accompany the epoxidation of cycloalkenes. Inhibition of reaction conditions and zeolite acidity selectively derive the various intermediates in the process.
subjectZeolites -- Research ; Manganese (Metal) -- Research;
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