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Observation of 239Pu Nuclear Magnetic Resonance

Nuclear magnetic resonance (NMR) spectroscopy and its spatially sensitive cousin, magnetic resonance imaging, have found widespread application in chemical and biological characterization studies. For the most part, these studies take advantage of the energy bifurcation manifested by hydrogen nuclei... Full description

Journal Title: Science May 18, 2012, Vol.336(6083), pp.901-904
Main Author: Yasuoka, H
Other Authors: Koutroulakis, G , Chudo, H , Richmond, S , Veirs, D , Smith, A , Bauer, E , Thompson, J , Jarvinen, G , Clark, D
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: ISSN: 00368075 ; E-ISSN: 10959203 ; DOI: 10.1126/science.1220801
Link: http://search.proquest.com/docview/1014146172/?pq-origsite=primo
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title: Observation of 239Pu Nuclear Magnetic Resonance
format: Article
creator:
  • Yasuoka, H
  • Koutroulakis, G
  • Chudo, H
  • Richmond, S
  • Veirs, D
  • Smith, A
  • Bauer, E
  • Thompson, J
  • Jarvinen, G
  • Clark, D
subjects:
  • Nuclear Magnetic Resonance–NMR
  • Spectrum Analysis
  • Atoms & Subatomic Particles
  • Plutonium
ispartof: Science, May 18, 2012, Vol.336(6083), pp.901-904
description: Nuclear magnetic resonance (NMR) spectroscopy and its spatially sensitive cousin, magnetic resonance imaging, have found widespread application in chemical and biological characterization studies. For the most part, these studies take advantage of the energy bifurcation manifested by hydrogen nuclei with oppositely directed spins in a strong magnetic field. More generally, many heavier elements manifest the same effect--including carbon-13, fluorine, and phosphorus. In theory, researchers have known for 50 years that plutonium nuclei have a net spin conducive to NMR. Yasuoka et al. (p. 901; see the Perspective by Albrecht-Schmitt ) have now at last observed the resonance of the Pu-239 isotope in a sample of plutonium dioxide. In principle, the spin-½ plutonium-239 (239Pu) nucleus should be active in nuclear magnetic resonance spectroscopy. However, its signal has eluded detection for the past 50 years. Here, we report observation of a 239Pu resonance from a solid sample of plutonium dioxide...
language: eng
source:
identifier: ISSN: 00368075 ; E-ISSN: 10959203 ; DOI: 10.1126/science.1220801
fulltext: no_fulltext
issn:
  • 00368075
  • 0036-8075
  • 10959203
  • 1095-9203
url: Link


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titleObservation of 239Pu Nuclear Magnetic Resonance
creatorYasuoka, H ; Koutroulakis, G ; Chudo, H ; Richmond, S ; Veirs, D ; Smith, A ; Bauer, E ; Thompson, J ; Jarvinen, G ; Clark, D
ispartofScience, May 18, 2012, Vol.336(6083), pp.901-904
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subjectNuclear Magnetic Resonance–NMR ; Spectrum Analysis ; Atoms & Subatomic Particles ; Plutonium
descriptionNuclear magnetic resonance (NMR) spectroscopy and its spatially sensitive cousin, magnetic resonance imaging, have found widespread application in chemical and biological characterization studies. For the most part, these studies take advantage of the energy bifurcation manifested by hydrogen nuclei with oppositely directed spins in a strong magnetic field. More generally, many heavier elements manifest the same effect--including carbon-13, fluorine, and phosphorus. In theory, researchers have known for 50 years that plutonium nuclei have a net spin conducive to NMR. Yasuoka et al. (p. 901; see the Perspective by Albrecht-Schmitt ) have now at last observed the resonance of the Pu-239 isotope in a sample of plutonium dioxide. In principle, the spin-½ plutonium-239 (239Pu) nucleus should be active in nuclear magnetic resonance spectroscopy. However, its signal has eluded detection for the past 50 years. Here, we report observation of a 239Pu resonance from a solid sample of plutonium dioxide...
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titleObservation of 239Pu Nuclear Magnetic Resonance
descriptionNuclear magnetic resonance (NMR) spectroscopy and its spatially sensitive cousin, magnetic resonance imaging, have found widespread application in chemical and biological characterization studies. For the most part, these studies take advantage of the energy bifurcation manifested by hydrogen nuclei with oppositely directed spins in a strong magnetic field. More generally, many heavier elements manifest the same effect--including carbon-13, fluorine, and phosphorus. In theory, researchers have known for 50 years that plutonium nuclei have a net spin conducive to NMR. Yasuoka et al. (p. 901; see the Perspective by Albrecht-Schmitt ) have now at last observed the resonance of the Pu-239 isotope in a sample of plutonium dioxide. In principle, the spin-½ plutonium-239 (239Pu) nucleus should be active in nuclear magnetic resonance spectroscopy. However, its signal has eluded detection for the past 50 years. Here, we report observation of a 239Pu resonance from a solid sample of plutonium dioxide...
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citationpf 901 pt 904 vol 336 issue 6083
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titleObservation of 239Pu Nuclear Magnetic Resonance
authorYasuoka, H ; Koutroulakis, G ; Chudo, H ; Richmond, S ; Veirs, D ; Smith, A ; Bauer, E ; Thompson, J ; Jarvinen, G ; Clark, D
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abstractNuclear magnetic resonance (NMR) spectroscopy and its spatially sensitive cousin, magnetic resonance imaging, have found widespread application in chemical and biological characterization studies. For the most part, these studies take advantage of the energy bifurcation manifested by hydrogen nuclei with oppositely directed spins in a strong magnetic field. More generally, many heavier elements manifest the same effect--including carbon-13, fluorine, and phosphorus. In theory, researchers have known for 50 years that plutonium nuclei have a net spin conducive to NMR. Yasuoka et al. (p. 901; see the Perspective by Albrecht-Schmitt ) have now at last observed the resonance of the Pu-239 isotope in a sample of plutonium dioxide. In principle, the spin-½ plutonium-239 (239Pu) nucleus should be active in nuclear magnetic resonance spectroscopy. However, its signal has eluded detection for the past 50 years. Here, we report observation of a 239Pu resonance from a solid sample of plutonium dioxide...
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pubThe American Association for the Advancement of Science
doi10.1126/science.1220801
urlhttp://search.proquest.com/docview/1014146172/
date2012-05-18