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Structural and spectroscopic characterization of a monomeric side-on manganese(IV) peroxo complex.

Gotcha: The binding and activation of oxygen by a manganese complex is reported. A PS sub(3) coordination sphere built around a manganese(I) center facilitates the isolation of a monomeric manganese(IV) peroxo complex that is stable at ambient temperature (see picture). The activation of molecular o... Full description

Journal Title: Angewandte Chemie (International ed. in English) May 29, 2012, Vol.51(22), pp.5427-5430
Main Author: Lee, Chien-Ming
Other Authors: Chuo, Chi-He , Chen, Ching-Hui , Hu, Cho-Chun , Chiang, Ming-Hsi , Tseng, Yu-Jan , Hu, Ching-Han , Lee, Gene-Hsiang
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201201735
Link: http://search.proquest.com/docview/1015754845/?pq-origsite=primo
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recordid: proquest1015754845
title: Structural and spectroscopic characterization of a monomeric side-on manganese(IV) peroxo complex.
format: Article
creator:
  • Lee, Chien-Ming
  • Chuo, Chi-He
  • Chen, Ching-Hui
  • Hu, Cho-Chun
  • Chiang, Ming-Hsi
  • Tseng, Yu-Jan
  • Hu, Ching-Han
  • Lee, Gene-Hsiang
subjects:
  • Electron Spin Resonance Spectroscopy–Chemistry
  • Manganese–Chemistry
  • Models, Molecular–Metabolism
  • Molecular Structure–Chemistry
  • Organometallic Compounds–Chemistry
  • Oxidation-Reduction–Chemistry
  • Oxygen–Chemistry
  • Spectrophotometry, Infrared–Chemistry
  • Spectrophotometry, Ultraviolet–Chemistry
  • Organometallic Compounds
  • Manganese
  • Oxygen
ispartof: Angewandte Chemie (International ed. in English), May 29, 2012, Vol.51(22), pp.5427-5430
description: Gotcha: The binding and activation of oxygen by a manganese complex is reported. A PS sub(3) coordination sphere built around a manganese(I) center facilitates the isolation of a monomeric manganese(IV) peroxo complex that is stable at ambient temperature (see picture). The activation of molecular oxygen is proposed via a manganese(II) intermediate with an empty site for the binding of the substrate.
language: eng
source:
identifier: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201201735
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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titleStructural and spectroscopic characterization of a monomeric side-on manganese(IV) peroxo complex.
creatorLee, Chien-Ming ; Chuo, Chi-He ; Chen, Ching-Hui ; Hu, Cho-Chun ; Chiang, Ming-Hsi ; Tseng, Yu-Jan ; Hu, Ching-Han ; Lee, Gene-Hsiang
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identifierE-ISSN: 1521-3773 ; DOI: 10.1002/anie.201201735
subjectElectron Spin Resonance Spectroscopy–Chemistry ; Manganese–Chemistry ; Models, Molecular–Metabolism ; Molecular Structure–Chemistry ; Organometallic Compounds–Chemistry ; Oxidation-Reduction–Chemistry ; Oxygen–Chemistry ; Spectrophotometry, Infrared–Chemistry ; Spectrophotometry, Ultraviolet–Chemistry ; Organometallic Compounds ; Manganese ; Oxygen
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descriptionGotcha: The binding and activation of oxygen by a manganese complex is reported. A PS sub(3) coordination sphere built around a manganese(I) center facilitates the isolation of a monomeric manganese(IV) peroxo complex that is stable at ambient temperature (see picture). The activation of molecular oxygen is proposed via a manganese(II) intermediate with an empty site for the binding of the substrate.
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titleStructural and spectroscopic characterization of a monomeric side-on manganese(IV) peroxo complex.
authorLee, Chien-Ming ; Chuo, Chi-He ; Chen, Ching-Hui ; Hu, Cho-Chun ; Chiang, Ming-Hsi ; Tseng, Yu-Jan ; Hu, Ching-Han ; Lee, Gene-Hsiang
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