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Catalytic C-H amination with aromatic amines.

Aniline joins the club: A [beta]-diketiminato copper(I) catalyst enables C--H amination of anilines employing low catalyst loadings to preclude oxidation to the diazene ArN==NAr (see scheme). Electron-poor anilines are particularly resistant towards diazene formation and participate in the amination... Full description

Journal Title: Angewandte Chemie (International ed. in English) June 25, 2012, Vol.51(26), pp.6488-6492
Main Author: Gephart, Raymond T
Other Authors: Huang, Daria L , Aguila, Mae Joanne B , Schmidt, Graham , Shahu, Andi , Warren, Timothy H
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; DOI: 1521-3773 ; DOI: 10.1002/anie.201201921
Link: http://search.proquest.com/docview/1021984661/?pq-origsite=primo
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recordid: proquest1021984661
title: Catalytic C-H amination with aromatic amines.
format: Article
creator:
  • Gephart, Raymond T
  • Huang, Daria L
  • Aguila, Mae Joanne B
  • Schmidt, Graham
  • Shahu, Andi
  • Warren, Timothy H
subjects:
  • Amination–Chemistry
  • Amines–Chemistry
  • Carbon–Chemistry
  • Catalysis–Chemistry
  • Hydrogen–Chemistry
  • Molecular Structure–Chemistry
  • Oxidation-Reduction–Chemistry
  • Amines
  • Carbon
  • Hydrogen
ispartof: Angewandte Chemie (International ed. in English), June 25, 2012, Vol.51(26), pp.6488-6492
description: Aniline joins the club: A [beta]-diketiminato copper(I) catalyst enables C--H amination of anilines employing low catalyst loadings to preclude oxidation to the diazene ArN==NAr (see scheme). Electron-poor anilines are particularly resistant towards diazene formation and participate in the amination of strong and unactivated C--H bonds. N-alkyl anilines also take part in C--H amination.
language: eng
source:
identifier: E-ISSN: 1521-3773 ; DOI: 1521-3773 ; DOI: 10.1002/anie.201201921
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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descriptionAniline joins the club: A [beta]-diketiminato copper(I) catalyst enables C--H amination of anilines employing low catalyst loadings to preclude oxidation to the diazene ArN==NAr (see scheme). Electron-poor anilines are particularly resistant towards diazene formation and participate in the amination of strong and unactivated C--H bonds. N-alkyl anilines also take part in C--H amination.
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