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Zirconium-metalloporphyrin PCN-222: mesoporous metal-organic frameworks with ultrahigh stability as biomimetic catalysts.

Biomimetic MOF: Extremely stable MOFs with different open metal sites and ultra-large 1D channels, PCN-222 (Fe, Mn, Co, Ni, Cu, and Zn), have been assembled with eight-connected Zr sub(6) clusters and redox-active metalloporphyrin motifs. PCN-222(Fe) shows peroxidase-like activity in aqueous solutio... Full description

Journal Title: Angewandte Chemie (International ed. in English) October 8, 2012, Vol.51(41), pp.10307-10310
Main Author: Feng, Dawei
Other Authors: Gu, Zhi-Yuan , Li, Jian-Rong , Jiang, Hai-Long , Wei, Zhangwen , Zhou, Hong-Cai
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201204475
Link: http://search.proquest.com/docview/1081871651/?pq-origsite=primo
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title: Zirconium-metalloporphyrin PCN-222: mesoporous metal-organic frameworks with ultrahigh stability as biomimetic catalysts.
format: Article
creator:
  • Feng, Dawei
  • Gu, Zhi-Yuan
  • Li, Jian-Rong
  • Jiang, Hai-Long
  • Wei, Zhangwen
  • Zhou, Hong-Cai
subjects:
  • Biomimetic Materials–Chemistry
  • Catalysis–Metabolism
  • Crystallography, X-Ray–Chemistry
  • Metalloporphyrins–Chemistry
  • Molecular Conformation–Chemistry
  • Oxidation-Reduction–Chemistry
  • Porosity–Chemistry
  • Zirconium–Chemistry
  • Metalloporphyrins
  • Zirconium
ispartof: Angewandte Chemie (International ed. in English), October 8, 2012, Vol.51(41), pp.10307-10310
description: Biomimetic MOF: Extremely stable MOFs with different open metal sites and ultra-large 1D channels, PCN-222 (Fe, Mn, Co, Ni, Cu, and Zn), have been assembled with eight-connected Zr sub(6) clusters and redox-active metalloporphyrin motifs. PCN-222(Fe) shows peroxidase-like activity in aqueous solution, exhibiting highly effective biomimetic oxidation on a number of substrates.
language: eng
source:
identifier: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201204475
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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titleZirconium-metalloporphyrin PCN-222: mesoporous metal-organic frameworks with ultrahigh stability as biomimetic catalysts.
creatorFeng, Dawei ; Gu, Zhi-Yuan ; Li, Jian-Rong ; Jiang, Hai-Long ; Wei, Zhangwen ; Zhou, Hong-Cai
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identifierE-ISSN: 1521-3773 ; DOI: 10.1002/anie.201204475
subjectBiomimetic Materials–Chemistry ; Catalysis–Metabolism ; Crystallography, X-Ray–Chemistry ; Metalloporphyrins–Chemistry ; Molecular Conformation–Chemistry ; Oxidation-Reduction–Chemistry ; Porosity–Chemistry ; Zirconium–Chemistry ; Metalloporphyrins ; Zirconium
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descriptionBiomimetic MOF: Extremely stable MOFs with different open metal sites and ultra-large 1D channels, PCN-222 (Fe, Mn, Co, Ni, Cu, and Zn), have been assembled with eight-connected Zr sub(6) clusters and redox-active metalloporphyrin motifs. PCN-222(Fe) shows peroxidase-like activity in aqueous solution, exhibiting highly effective biomimetic oxidation on a number of substrates.
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