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Oxidative geminal functionalization of organoboron compounds.

Excellent tolerance: Stable acylboronates equipped with N-methyliminodiacetyl (MIDA) boryl groups ([B]) were prepared by using a sequence of oxidative manipulations at the boron-bound carbon center (green in scheme). Chemoselective transformations of these acylated organoboron building blocks yielde... Full description

Journal Title: Angewandte Chemie (International ed. in English) October 29, 2012, Vol.51(44), pp.11092-11096
Main Author: He, Zhi
Other Authors: Trinchera, Piera , Adachi, Shinya , St Denis, Jeffrey D , Yudin, Andrei K
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201206501
Link: http://search.proquest.com/docview/1115526019/?pq-origsite=primo
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recordid: proquest1115526019
title: Oxidative geminal functionalization of organoboron compounds.
format: Article
creator:
  • He, Zhi
  • Trinchera, Piera
  • Adachi, Shinya
  • St Denis, Jeffrey D
  • Yudin, Andrei K
subjects:
  • Boronic Acids–Chemical Synthesis
  • Crystallography, X-Ray–Chemistry
  • Models, Molecular–Chemistry
  • Molecular Structure–Chemistry
  • Oxidation-Reduction–Chemistry
  • Boronic Acids
ispartof: Angewandte Chemie (International ed. in English), October 29, 2012, Vol.51(44), pp.11092-11096
description: Excellent tolerance: Stable acylboronates equipped with N-methyliminodiacetyl (MIDA) boryl groups ([B]) were prepared by using a sequence of oxidative manipulations at the boron-bound carbon center (green in scheme). Chemoselective transformations of these acylated organoboron building blocks yielded a range of multifunctionalized boron derivatives and supplied access to valuable borylated heterocycles (see scheme).
language: eng
source:
identifier: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201206501
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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descriptionExcellent tolerance: Stable acylboronates equipped with N-methyliminodiacetyl (MIDA) boryl groups ([B]) were prepared by using a sequence of oxidative manipulations at the boron-bound carbon center (green in scheme). Chemoselective transformations of these acylated organoboron building blocks yielded a range of multifunctionalized boron derivatives and supplied access to valuable borylated heterocycles (see scheme).
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