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Fine-tuning pore size by shifting coordination sites of ligands and surface polarization of metal-organic frameworks to sharply enhance the selectivity for CO2.

The coordination sites of ligands were shifted to fine-tune the pore size and polarization of the inner surface of metal-organic frameworks with uncoordinated nitrogen atoms. The findings demonstrated the valuable characteristics of the NJU-Bai8 which exhibits high uptake of C[O.sub.2] and good C[O.... Full description

Journal Title: Journal of the American Chemical Society January 16, 2013, Vol.135(2), pp.562-565
Main Author: Du, Liting
Other Authors: Lu, Zhiyong , Zheng, Kaiyuan , Wang, Junyi , Zheng, Xin , Pan, Yi , You, Xiaozeng , Bai, Junfeng
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1520-5126 ; DOI: 1520-5126 ; DOI: 10.1021/ja309992a
Link: http://search.proquest.com/docview/1273576636/?pq-origsite=primo
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title: Fine-tuning pore size by shifting coordination sites of ligands and surface polarization of metal-organic frameworks to sharply enhance the selectivity for CO2.
format: Article
creator:
  • Du, Liting
  • Lu, Zhiyong
  • Zheng, Kaiyuan
  • Wang, Junyi
  • Zheng, Xin
  • Pan, Yi
  • You, Xiaozeng
  • Bai, Junfeng
subjects:
  • Carbon Dioxide -- Structure
  • Carbon Dioxide -- Chemical Properties
  • Isophthalic Acid -- Chemical Properties
  • Polarization (Electricity) -- Analysis
  • Surface Energy -- Measurement
ispartof: Journal of the American Chemical Society, January 16, 2013, Vol.135(2), pp.562-565
description: The coordination sites of ligands were shifted to fine-tune the pore size and polarization of the inner surface of metal-organic frameworks with uncoordinated nitrogen atoms. The findings demonstrated the valuable characteristics of the NJU-Bai8 which exhibits high uptake of C[O.sub.2] and good C[O.sub.2]/C[H.sub.4] selectivity at high pressure in the purification of natural gases.
language: eng
source:
identifier: E-ISSN: 1520-5126 ; DOI: 1520-5126 ; DOI: 10.1021/ja309992a
fulltext: no_fulltext
issn:
  • 15205126
  • 1520-5126
url: Link


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titleFine-tuning pore size by shifting coordination sites of ligands and surface polarization of metal-organic frameworks to sharply enhance the selectivity for CO2.
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descriptionThe coordination sites of ligands were shifted to fine-tune the pore size and polarization of the inner surface of metal-organic frameworks with uncoordinated nitrogen atoms. The findings demonstrated the valuable characteristics of the NJU-Bai8 which exhibits high uptake of C[O.sub.2] and good C[O.sub.2]/C[H.sub.4] selectivity at high pressure in the purification of natural gases.
subjectCarbon Dioxide -- Structure ; Carbon Dioxide -- Chemical Properties ; Isophthalic Acid -- Chemical Properties ; Polarization (Electricity) -- Analysis ; Surface Energy -- Measurement;
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