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Photocatalytic oxidation of organic compounds in water by using ruthenium(II)-pyridylamine complexes as catalysts with high efficiency and selectivity.

The photocatalytic oxidation of organic substrates such as alcohols was conducted in the presence of Ru super(II)-aqua complexes as oxidation catalysts, [Ru super(II)(bpy) sub(3)] super(2+) as a photosensitizer and electron mediator, and a Co super(III) complex as a sacrificial oxidant (see scheme).... Full description

Journal Title: Chemistry (Weinheim an der Bergstrasse Germany), January 28, 2013, Vol.19(5), pp.1563-1567
Main Author: Ohzu, Shingo
Other Authors: Ishizuka, Tomoya , Hirai, Yuichirou , Fukuzumi, Shunichi , Kojima, Takahiko
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3765 ; DOI: 1521-3765 ; DOI: 10.1002/chem.201203430
Link: http://search.proquest.com/docview/1273628105/?pq-origsite=primo
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title: Photocatalytic oxidation of organic compounds in water by using ruthenium(II)-pyridylamine complexes as catalysts with high efficiency and selectivity.
format: Article
creator:
  • Ohzu, Shingo
  • Ishizuka, Tomoya
  • Hirai, Yuichirou
  • Fukuzumi, Shunichi
  • Kojima, Takahiko
subjects:
  • Catalysis–Chemistry
  • Organometallic Compounds–Chemistry
  • Oxidation-Reduction–Chemistry
  • Photochemistry–Chemistry
  • Ruthenium–Chemistry
  • Water–Chemistry
  • Organometallic Compounds
  • Water
  • Ruthenium
ispartof: Chemistry (Weinheim an der Bergstrasse, Germany), January 28, 2013, Vol.19(5), pp.1563-1567
description: The photocatalytic oxidation of organic substrates such as alcohols was conducted in the presence of Ru super(II)-aqua complexes as oxidation catalysts, [Ru super(II)(bpy) sub(3)] super(2+) as a photosensitizer and electron mediator, and a Co super(III) complex as a sacrificial oxidant (see scheme). The catalytic systems exhibited high efficiency to achieve turnover numbers of over 8000.
language: eng
source:
identifier: E-ISSN: 1521-3765 ; DOI: 1521-3765 ; DOI: 10.1002/chem.201203430
fulltext: fulltext
issn:
  • 15213765
  • 1521-3765
url: Link


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descriptionThe photocatalytic oxidation of organic substrates such as alcohols was conducted in the presence of Ru super(II)-aqua complexes as oxidation catalysts, [Ru super(II)(bpy) sub(3)] super(2+) as a photosensitizer and electron mediator, and a Co super(III) complex as a sacrificial oxidant (see scheme). The catalytic systems exhibited high efficiency to achieve turnover numbers of over 8000.
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