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Direct functionalization of tetrahydrofuran and 1,4-dioxane: nickel-catalyzed oxidative C(sp3)-H arylation.

CHoose nickel: The nickel-catalyzed oxidative arylation of C(sp super(3))--H bonds has been achieved. Several substituted arylboronic acids and various C(sp super(3))--H bonds were found to be suitable substrates for this novel transformation, which is likely to proceed through a radical pathway. Th... Full description

Journal Title: Angewandte Chemie (International ed. in English) April 15, 2013, Vol.52(16), pp.4453-4456
Main Author: Liu, Dong
Other Authors: Liu, Chao , Li, Heng , Lei, Aiwen
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; DOI: 1521-3773 ; DOI: 10.1002/anie.201300459
Link: http://search.proquest.com/docview/1326731267/?pq-origsite=primo
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title: Direct functionalization of tetrahydrofuran and 1,4-dioxane: nickel-catalyzed oxidative C(sp3)-H arylation.
format: Article
creator:
  • Liu, Dong
  • Liu, Chao
  • Li, Heng
  • Lei, Aiwen
subjects:
  • Catalysis–Chemistry
  • Dioxanes–Chemistry
  • Furans–Chemistry
  • Molecular Structure–Chemistry
  • Nickel–Chemistry
  • Oxidation-Reduction–Chemistry
  • Dioxanes
  • Furans
  • Tetrahydrofuran
  • Nickel
  • 1,4-Dioxane
ispartof: Angewandte Chemie (International ed. in English), April 15, 2013, Vol.52(16), pp.4453-4456
description: CHoose nickel: The nickel-catalyzed oxidative arylation of C(sp super(3))--H bonds has been achieved. Several substituted arylboronic acids and various C(sp super(3))--H bonds were found to be suitable substrates for this novel transformation, which is likely to proceed through a radical pathway. This method allows the introduction of simple ether derivatives to construct [alpha]-arylated ethers. FG=functional group.
language: eng
source:
identifier: E-ISSN: 1521-3773 ; DOI: 1521-3773 ; DOI: 10.1002/anie.201300459
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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titleDirect functionalization of tetrahydrofuran and 1,4-dioxane: nickel-catalyzed oxidative C(sp3)-H arylation.
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subjectCatalysis–Chemistry ; Dioxanes–Chemistry ; Furans–Chemistry ; Molecular Structure–Chemistry ; Nickel–Chemistry ; Oxidation-Reduction–Chemistry ; Dioxanes ; Furans ; Tetrahydrofuran ; Nickel ; 1,4-Dioxane
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descriptionCHoose nickel: The nickel-catalyzed oxidative arylation of C(sp super(3))--H bonds has been achieved. Several substituted arylboronic acids and various C(sp super(3))--H bonds were found to be suitable substrates for this novel transformation, which is likely to proceed through a radical pathway. This method allows the introduction of simple ether derivatives to construct [alpha]-arylated ethers. FG=functional group.
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