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Copper-catalyzed oxidative benzylarylation of acrylamides by benzylic C-H bond functionalization for the synthesis of oxindoles.

Radically changing benzyls: An efficient method for the benzylarylation of activated alkenes has been developed through a copper-catalyzed tandem radical addition/cyclization strategy (see scheme). This oxidative coupling between acrylamides and benzylic hydrocarbons provides access to diverse alkyl... Full description

Journal Title: Chemistry (Weinheim an der Bergstrasse Germany), September 23, 2013, Vol.19(39), pp.12970-12973
Main Author: Zhou, Shi-Liu
Other Authors: Guo, Li-Na , Wang, Hua , Duan, Xin-Hua
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3765 ; DOI: 1521-3765 ; DOI: 10.1002/chem.201302139
Link: http://search.proquest.com/docview/1434744544/?pq-origsite=primo
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title: Copper-catalyzed oxidative benzylarylation of acrylamides by benzylic C-H bond functionalization for the synthesis of oxindoles.
format: Article
creator:
  • Zhou, Shi-Liu
  • Guo, Li-Na
  • Wang, Hua
  • Duan, Xin-Hua
subjects:
  • Acrylamides–Chemistry
  • Benzyl Compounds–Chemistry
  • Catalysis–Chemistry
  • Copper–Chemistry
  • Cyclization–Chemical Synthesis
  • Cycloparaffins–Chemistry
  • Indoles–Chemistry
  • Oxidation-Reduction–Chemistry
  • Oxidative Coupling–Chemistry
  • Acrylamides
  • Benzyl Compounds
  • Cycloparaffins
  • Indoles
  • 2-Oxindole
  • Copper
  • Activated Alkenes
  • Benzylarylation
  • Copper
  • Oxindoles
  • Radical Addition
ispartof: Chemistry (Weinheim an der Bergstrasse, Germany), September 23, 2013, Vol.19(39), pp.12970-12973
description: Radically changing benzyls: An efficient method for the benzylarylation of activated alkenes has been developed through a copper-catalyzed tandem radical addition/cyclization strategy (see scheme). This oxidative coupling between acrylamides and benzylic hydrocarbons provides access to diverse alkyl-substituted oxindoles in good to excellent yields. A variety of functional groups were tolerated in this transformation (TBPB = tert-butylperoxy benzoate).
language: eng
source:
identifier: E-ISSN: 1521-3765 ; DOI: 1521-3765 ; DOI: 10.1002/chem.201302139
fulltext: fulltext
issn:
  • 15213765
  • 1521-3765
url: Link


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titleCopper-catalyzed oxidative benzylarylation of acrylamides by benzylic C-H bond functionalization for the synthesis of oxindoles.
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ispartofChemistry (Weinheim an der Bergstrasse, Germany), September 23, 2013, Vol.19(39), pp.12970-12973
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subjectAcrylamides–Chemistry ; Benzyl Compounds–Chemistry ; Catalysis–Chemistry ; Copper–Chemistry ; Cyclization–Chemical Synthesis ; Cycloparaffins–Chemistry ; Indoles–Chemistry ; Oxidation-Reduction–Chemistry ; Oxidative Coupling–Chemistry ; Acrylamides ; Benzyl Compounds ; Cycloparaffins ; Indoles ; 2-Oxindole ; Copper ; Activated Alkenes ; Benzylarylation ; Copper ; Oxindoles ; Radical Addition
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descriptionRadically changing benzyls: An efficient method for the benzylarylation of activated alkenes has been developed through a copper-catalyzed tandem radical addition/cyclization strategy (see scheme). This oxidative coupling between acrylamides and benzylic hydrocarbons provides access to diverse alkyl-substituted oxindoles in good to excellent yields. A variety of functional groups were tolerated in this transformation (TBPB = tert-butylperoxy benzoate).
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titleCopper-catalyzed oxidative benzylarylation of acrylamides by benzylic C-H bond functionalization for the synthesis of oxindoles.
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