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Visible light-mediated C-H difluoromethylation of electron-rich heteroarenes.

A novel method for visible-light photoredox-catalyzed difluoromethylation of electron-rich N-, O-, and S-containingheteroarenes under mild reaction conditions is developed. Mechanistic investigation indicates that the net C–H difluoromethylation proceeds through an electrophilic radical-type pathway... Full description

Journal Title: Organic letters June 6, 2014, Vol.16(11), pp.2958-2961
Main Author: Su, Yi-Ming
Other Authors: Hou, Yu , Yin, Feng , Xu, Yue-Ming , Li, Yan , Zheng, Xiaoqi , Wang, Xi-Sheng
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1523-7052 ; DOI: 10.1021/ol501094z
Link: http://search.proquest.com/docview/1534100154/?pq-origsite=primo
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title: Visible light-mediated C-H difluoromethylation of electron-rich heteroarenes.
format: Article
creator:
  • Su, Yi-Ming
  • Hou, Yu
  • Yin, Feng
  • Xu, Yue-Ming
  • Li, Yan
  • Zheng, Xiaoqi
  • Wang, Xi-Sheng
subjects:
  • Catalysis–Chemical Synthesis
  • Electrons–Chemistry
  • Heterocyclic Compounds–Chemical Synthesis
  • Hydrocarbons, Fluorinated–Chemistry
  • Hydrogen Bonding–Chemistry
  • Light–Chemistry
  • Methylation–Chemistry
  • Molecular Structure–Chemistry
  • Photochemical Processes–Chemistry
  • Heterocyclic Compounds
  • Hydrocarbons, Fluorinated
ispartof: Organic letters, June 6, 2014, Vol.16(11), pp.2958-2961
description: A novel method for visible-light photoredox-catalyzed difluoromethylation of electron-rich N-, O-, and S-containingheteroarenes under mild reaction conditions is developed. Mechanistic investigation indicates that the net C–H difluoromethylation proceeds through an electrophilic radical-type pathway.
language: eng
source:
identifier: E-ISSN: 1523-7052 ; DOI: 10.1021/ol501094z
fulltext: fulltext
issn:
  • 15237052
  • 1523-7052
url: Link


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titleVisible light-mediated C-H difluoromethylation of electron-rich heteroarenes.
creatorSu, Yi-Ming ; Hou, Yu ; Yin, Feng ; Xu, Yue-Ming ; Li, Yan ; Zheng, Xiaoqi ; Wang, Xi-Sheng
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ispartofOrganic letters, June 6, 2014, Vol.16(11), pp.2958-2961
identifierE-ISSN: 1523-7052 ; DOI: 10.1021/ol501094z
subjectCatalysis–Chemical Synthesis ; Electrons–Chemistry ; Heterocyclic Compounds–Chemical Synthesis ; Hydrocarbons, Fluorinated–Chemistry ; Hydrogen Bonding–Chemistry ; Light–Chemistry ; Methylation–Chemistry ; Molecular Structure–Chemistry ; Photochemical Processes–Chemistry ; Heterocyclic Compounds ; Hydrocarbons, Fluorinated
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descriptionA novel method for visible-light photoredox-catalyzed difluoromethylation of electron-rich N-, O-, and S-containingheteroarenes under mild reaction conditions is developed. Mechanistic investigation indicates that the net C–H difluoromethylation proceeds through an electrophilic radical-type pathway.
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titleVisible light-mediated C-H difluoromethylation of electron-rich heteroarenes.
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