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Metal-free oxidative C(sp(3))-H bond functionalization of alkanes and alkylation-initiated radical 1,2-aryl migration in α,α-diaryl allylic alcohols.

An oxidative C(sp super(3))-H bond functionalization of alkanes and alkylation-initiated radical 1,2-aryl migration in alpha , alpha -diaryl allylic alcohols using di-tert-butyl peroxide (DTBP) as the oxidant was established, which tolerates a wide range of simple alkane substrates and alpha , alpha... Full description

Journal Title: Chemical communications (Cambridge England), January 11, 2015, Vol.51(3), pp.599-602
Main Author: Zhao, Jincan
Other Authors: Fang, Hong , Song, Ruichun , Zhou, Jie , Han, Jianlin , Pan, Yi
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1364-548X ; DOI: 1364-548X ; DOI: 10.1039/c4cc07654k
Link: http://search.proquest.com/docview/1635001713/?pq-origsite=primo
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recordid: proquest1635001713
title: Metal-free oxidative C(sp(3))-H bond functionalization of alkanes and alkylation-initiated radical 1,2-aryl migration in α,α-diaryl allylic alcohols.
format: Article
creator:
  • Zhao, Jincan
  • Fang, Hong
  • Song, Ruichun
  • Zhou, Jie
  • Han, Jianlin
  • Pan, Yi
subjects:
  • Alkanes–Chemistry
  • Alkylation–Chemistry
  • Molecular Structure–Chemistry
  • Oxidation-Reduction–Chemistry
  • Propanols–Chemistry
  • Alkanes
  • Propanols
  • Allyl Alcohol
ispartof: Chemical communications (Cambridge, England), January 11, 2015, Vol.51(3), pp.599-602
description: An oxidative C(sp super(3))-H bond functionalization of alkanes and alkylation-initiated radical 1,2-aryl migration in alpha , alpha -diaryl allylic alcohols using di-tert-butyl peroxide (DTBP) as the oxidant was established, which tolerates a wide range of simple alkane substrates and alpha , alpha -diaryl allylic alcohols for direct preparation of alpha -aryl- beta -alkylated carbonyl ketones.
language: eng
source:
identifier: E-ISSN: 1364-548X ; DOI: 1364-548X ; DOI: 10.1039/c4cc07654k
fulltext: fulltext
issn:
  • 1364548X
  • 1364-548X
url: Link


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titleMetal-free oxidative C(sp(3))-H bond functionalization of alkanes and alkylation-initiated radical 1,2-aryl migration in α,α-diaryl allylic alcohols.
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