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Asymmetric Synthesis of [beta]-Amino Nitriles through a Sc super(III)-Catalyzed Three-Component Mannich Reaction of Silyl Ketene Imines

A range of [beta]-amino nitriles containing contiguous tertiary and quaternary stereogenic carbon centers were synthesized by using the title reaction. The reaction was catalyzed by a chiral N,N'-dioxide scandium(III) complex under mild reaction conditions. Based on experimental...

Journal Title: Angewandte Chemie (International Edition) Mar 2013, Vol.52(12), pp.3473-3477
Main Author: Zhao, Jiannan
Other Authors: Liu, Xiaohua , Luo, Weiwei , Xie, Mingsheng , Lin, Lili , Feng, Xiaoming
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: ISSN: 1433-7851 ; E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201209093
Link: http://search.proquest.com/docview/1700990497/?pq-origsite=primo
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title: Asymmetric Synthesis of [beta]-Amino Nitriles through a Sc super(III)-Catalyzed Three-Component Mannich Reaction of Silyl Ketene Imines
format: Article
creator:
  • Zhao, Jiannan
  • Liu, Xiaohua
  • Luo, Weiwei
  • Xie, Mingsheng
  • Lin, Lili
  • Feng, Xiaoming
subjects:
  • Nitriles
  • Carbon
  • Asymmetry
  • Origins
  • Ketenes
  • Imines
  • Synthesis
  • Analysis (MD)
  • Chemical Analysis (Ep)
  • Chemical Analysis (Ed)
  • Chemical Analysis (EC)
  • Asymmetric Catalysis
  • Mannich Reaction
  • Silyl Ketene Imine
  • Multicomponent Reactions
  • [Beta]-Amino Nitrile
ispartof: Angewandte Chemie (International Edition), Mar 2013, Vol.52(12), pp.3473-3477
description: A range of [beta]-amino nitriles containing contiguous tertiary and quaternary stereogenic carbon centers were synthesized by using the title reaction. The reaction was catalyzed by a chiral N,N'-dioxide scandium(III) complex under mild reaction conditions. Based on experimental...
language: eng
source:
identifier: ISSN: 1433-7851 ; E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201209093
fulltext: fulltext
issn:
  • 14337851
  • 1433-7851
  • 15213773
  • 1521-3773
url: Link


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titleAsymmetric Synthesis of [beta]-Amino Nitriles through a Sc super(III)-Catalyzed Three-Component Mannich Reaction of Silyl Ketene Imines
creatorZhao, Jiannan ; Liu, Xiaohua ; Luo, Weiwei ; Xie, Mingsheng ; Lin, Lili ; Feng, Xiaoming
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subjectNitriles ; Carbon ; Asymmetry ; Origins ; Ketenes ; Imines ; Synthesis ; Analysis (MD) ; Chemical Analysis (Ep) ; Chemical Analysis (Ed) ; Chemical Analysis (EC) ; Asymmetric Catalysis ; Mannich Reaction ; Silyl Ketene Imine ; Multicomponent Reactions ; [Beta]-Amino Nitrile
descriptionA range of [beta]-amino nitriles containing contiguous tertiary and quaternary stereogenic carbon centers were synthesized by using the title reaction. The reaction was catalyzed by a chiral N,N'-dioxide scandium(III) complex under mild reaction conditions. Based on experimental...
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titleAsymmetric Synthesis of [beta]-Amino Nitriles through a Sc super(III)-Catalyzed Three-Component Mannich Reaction of Silyl Ketene Imines
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titleAsymmetric Synthesis of [beta]-Amino Nitriles through a Sc super(III)-Catalyzed Three-Component Mannich Reaction of Silyl Ketene Imines
authorZhao, Jiannan ; Liu, Xiaohua ; Luo, Weiwei ; Xie, Mingsheng ; Lin, Lili ; Feng, Xiaoming
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abstractA range of [beta]-amino nitriles containing contiguous tertiary and quaternary stereogenic carbon centers were synthesized by using the title reaction. The reaction was catalyzed by a chiral N,N'-dioxide scandium(III) complex under mild reaction conditions. Based on experimental...
doi10.1002/anie.201209093
urlhttp://search.proquest.com/docview/1700990497/
date2013-03-18