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Deep Desulfurization of Fuels by Extraction with 4-Dimethylaminopyridinium-Based Ionic Liquids

In this work, three 4-dimethylaminopyridinium-based ionic liquids (ILs), N-ethyl-4-dimethylaminopyridinium dicyanamide ([C sub(2) super(4)DMAPy][N(CN) sub(2)]), N-butyl-4-dimethylaminopyridinium dicyanamide ([C sub(4) super(4)DMAPy][N(CN) sub(2)]) and N-hexyl-4-dimethylaminopyridinium dicyanamide ([... Full description

Journal Title: Energy & Fuels Aug 15, 2013, Vol.27(8), pp.4617-4623-4617-4623
Main Author: Wang, Qianli
Other Authors: Lei, Lecheng , Zhu, Jingke , Yang, Bin , Li, Zhongjian
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: ISSN: 0887-0624 ; E-ISSN: 1520-5029 ; DOI: 10.1021/ef401015c
Link: http://search.proquest.com/docview/1701090888/?pq-origsite=primo
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title: Deep Desulfurization of Fuels by Extraction with 4-Dimethylaminopyridinium-Based Ionic Liquids
format: Article
creator:
  • Wang, Qianli
  • Lei, Lecheng
  • Zhu, Jingke
  • Yang, Bin
  • Li, Zhongjian
subjects:
  • Sulfur
  • Partitions
  • Solubility
  • Extraction
  • Gasoline
  • Fuels
  • Diesel
  • Coefficients
ispartof: Energy & Fuels, Aug 15, 2013, Vol.27(8), pp.4617-4623-4617-4623
description: In this work, three 4-dimethylaminopyridinium-based ionic liquids (ILs), N-ethyl-4-dimethylaminopyridinium dicyanamide ([C sub(2) super(4)DMAPy][N(CN) sub(2)]), N-butyl-4-dimethylaminopyridinium dicyanamide ([C sub(4) super(4)DMAPy][N(CN) sub(2)]) and N-hexyl-4-dimethylaminopyridinium dicyanamide ([C sub(6) super(4)DMAPy][N(CN) sub(2)]), were synthesized and then demonstrated to be efficient for aromatic sulfur compounds extraction from fuels. The mutual solubility evaluating results indicated that 4-dimethylaminopyridinium-based ILs hardly dissolved in the fuels, while the solubility of 97 super(#) gasoline in ILs varies from 7.0 wt % for [C sub(2) super(4)DMAPy][N(CN) sub(2)] to 12.4 wt % for [C sub(6) super(4)DMAPy][N(CN) sub(2)] and the solubility of 0 super(#) diesel in ILs varies from 6.7 wt % for [C sub(2) super(4)DMAPy][N(CN) sub(2)] to 9.7 wt % for [C sub(6) super(4)DMAPy][N(CN) sub(2)]. Also, the sulfur partition coefficient was evaluated. In the case of...
language: eng
source:
identifier: ISSN: 0887-0624 ; E-ISSN: 1520-5029 ; DOI: 10.1021/ef401015c
fulltext: fulltext
issn:
  • 08870624
  • 0887-0624
  • 15205029
  • 1520-5029
url: Link


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titleDeep Desulfurization of Fuels by Extraction with 4-Dimethylaminopyridinium-Based Ionic Liquids
creatorWang, Qianli ; Lei, Lecheng ; Zhu, Jingke ; Yang, Bin ; Li, Zhongjian
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ispartofEnergy & Fuels, Aug 15, 2013, Vol.27(8), pp.4617-4623-4617-4623
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subjectSulfur ; Partitions ; Solubility ; Extraction ; Gasoline ; Fuels ; Diesel ; Coefficients
descriptionIn this work, three 4-dimethylaminopyridinium-based ionic liquids (ILs), N-ethyl-4-dimethylaminopyridinium dicyanamide ([C sub(2) super(4)DMAPy][N(CN) sub(2)]), N-butyl-4-dimethylaminopyridinium dicyanamide ([C sub(4) super(4)DMAPy][N(CN) sub(2)]) and N-hexyl-4-dimethylaminopyridinium dicyanamide ([C sub(6) super(4)DMAPy][N(CN) sub(2)]), were synthesized and then demonstrated to be efficient for aromatic sulfur compounds extraction from fuels. The mutual solubility evaluating results indicated that 4-dimethylaminopyridinium-based ILs hardly dissolved in the fuels, while the solubility of 97 super(#) gasoline in ILs varies from 7.0 wt % for [C sub(2) super(4)DMAPy][N(CN) sub(2)] to 12.4 wt % for [C sub(6) super(4)DMAPy][N(CN) sub(2)] and the solubility of 0 super(#) diesel in ILs varies from 6.7 wt % for [C sub(2) super(4)DMAPy][N(CN) sub(2)] to 9.7 wt % for [C sub(6) super(4)DMAPy][N(CN) sub(2)]. Also, the sulfur partition coefficient was evaluated. In the case of...
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titleDeep Desulfurization of Fuels by Extraction with 4-Dimethylaminopyridinium-Based Ionic Liquids
descriptionIn this work, three 4-dimethylaminopyridinium-based ionic liquids (ILs), N-ethyl-4-dimethylaminopyridinium dicyanamide ([C sub(2) super(4)DMAPy][N(CN) sub(2)]), N-butyl-4-dimethylaminopyridinium dicyanamide ([C sub(4) super(4)DMAPy][N(CN) sub(2)]) and N-hexyl-4-dimethylaminopyridinium dicyanamide ([C sub(6) super(4)DMAPy][N(CN) sub(2)]), were synthesized and then demonstrated to be efficient for aromatic sulfur compounds extraction from fuels. The mutual solubility evaluating results indicated that 4-dimethylaminopyridinium-based ILs hardly dissolved in the fuels, while the solubility of 97 super(#) gasoline in ILs varies from 7.0 wt % for [C sub(2) super(4)DMAPy][N(CN) sub(2)] to 12.4 wt % for [C sub(6) super(4)DMAPy][N(CN) sub(2)] and the solubility of 0 super(#) diesel in ILs varies from 6.7 wt % for [C sub(2) super(4)DMAPy][N(CN) sub(2)] to 9.7 wt % for [C sub(6) super(4)DMAPy][N(CN) sub(2)]. Also, the sulfur partition coefficient was evaluated. In the case of...
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titleDeep Desulfurization of Fuels by Extraction with 4-Dimethylaminopyridinium-Based Ionic Liquids
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abstractIn this work, three 4-dimethylaminopyridinium-based ionic liquids (ILs), N-ethyl-4-dimethylaminopyridinium dicyanamide ([C sub(2) super(4)DMAPy][N(CN) sub(2)]), N-butyl-4-dimethylaminopyridinium dicyanamide ([C sub(4) super(4)DMAPy][N(CN) sub(2)]) and N-hexyl-4-dimethylaminopyridinium dicyanamide ([C sub(6) super(4)DMAPy][N(CN) sub(2)]), were synthesized and then demonstrated to be efficient for aromatic sulfur compounds extraction from fuels. The mutual solubility evaluating results indicated that 4-dimethylaminopyridinium-based ILs hardly dissolved in the fuels, while the solubility of 97 super(#) gasoline in ILs varies from 7.0 wt % for [C sub(2) super(4)DMAPy][N(CN) sub(2)] to 12.4 wt % for [C sub(6) super(4)DMAPy][N(CN) sub(2)] and the solubility of 0 super(#) diesel in ILs varies from 6.7 wt % for [C sub(2) super(4)DMAPy][N(CN) sub(2)] to 9.7 wt % for [C sub(6) super(4)DMAPy][N(CN) sub(2)]. Also, the sulfur partition coefficient was evaluated. In the case of...
doi10.1021/ef401015c
urlhttp://search.proquest.com/docview/1701090888/
date2013-08-15