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Singlet Oxygen-Engaged Selective Photo-Oxidation over Pt Nanocrystals/Porphyrinic MOF: The Roles of Photothermal Effect and Pt Electronic State.

Pt/PCN-224(M) composites by integration of Pt nanocrystals and porphyrinic metaluorganic frameworks (MOFs), PCN-224(M), are designed and synthesized. The composites exhibit excellent catalytic performance in the photo-oxidation of aromatic alcohols by 1 atm O2 at ambient temperature, based on a syne... Full description

Journal Title: Journal of the American Chemical Society February 8, 2017, Vol.139(5), pp.2035-2044
Main Author: Chen, Yu-Zhen
Other Authors: Wang, Zhiyong U , Wang, Hengwei , Lu, Junling , Yu, Shu-Hong , Jiang, Hai-Long
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1520-5126 ; DOI: 1520-5126 ; DOI: 10.1021/jacs.6b12074
Link: http://search.proquest.com/docview/1861582358/?pq-origsite=primo
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title: Singlet Oxygen-Engaged Selective Photo-Oxidation over Pt Nanocrystals/Porphyrinic MOF: The Roles of Photothermal Effect and Pt Electronic State.
format: Article
creator:
  • Chen, Yu-Zhen
  • Wang, Zhiyong U
  • Wang, Hengwei
  • Lu, Junling
  • Yu, Shu-Hong
  • Jiang, Hai-Long
subjects:
  • Chemical Synthesis – Usage
  • Catalysis – Usage
  • Platinum – Chemical Properties
  • Oxidation-Reduction Reactions – Usage
  • Aromatic Alcohols – Chemical Properties
ispartof: Journal of the American Chemical Society, February 8, 2017, Vol.139(5), pp.2035-2044
description: Pt/PCN-224(M) composites by integration of Pt nanocrystals and porphyrinic metaluorganic frameworks (MOFs), PCN-224(M), are designed and synthesized. The composites exhibit excellent catalytic performance in the photo-oxidation of aromatic alcohols by 1 atm O2 at ambient temperature, based on a synergetic photothermal effect and singlet oxygen production.This is an unprecedented report on singlet oxygen-engaged selective oxidation of aromatic alcohols to aldehydes and also the first report on photothermal effect of MOFs.
language: eng
source:
identifier: E-ISSN: 1520-5126 ; DOI: 1520-5126 ; DOI: 10.1021/jacs.6b12074
fulltext: no_fulltext
issn:
  • 15205126
  • 1520-5126
url: Link


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titleSinglet Oxygen-Engaged Selective Photo-Oxidation over Pt Nanocrystals/Porphyrinic MOF: The Roles of Photothermal Effect and Pt Electronic State.
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descriptionPt/PCN-224(M) composites by integration of Pt nanocrystals and porphyrinic metaluorganic frameworks (MOFs), PCN-224(M), are designed and synthesized. The composites exhibit excellent catalytic performance in the photo-oxidation of aromatic alcohols by 1 atm O2 at ambient temperature, based on a synergetic photothermal effect and singlet oxygen production.This is an unprecedented report on singlet oxygen-engaged selective oxidation of aromatic alcohols to aldehydes and also the first report on photothermal effect of MOFs.
subjectChemical Synthesis – Usage ; Catalysis – Usage ; Platinum – Chemical Properties ; Oxidation-Reduction Reactions – Usage ; Aromatic Alcohols – Chemical Properties;
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