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A biomimetic iron catalyst for the epoxidation of olefins with molecular oxygen at room temperature.

It's no sacrifice: A bio‐inspired iron system, in which a β‐keto ester serves as a sacrificial cosubstrate, readily epoxidizes olefins under ambient conditions with air. Aromatic olefins are oxidized in high yields with excellent chemoselectivity. Mechanistic investigations point out substantial dif... Full description

Journal Title: Angewandte Chemie (International ed. in English) February 7, 2011, Vol.50(6), pp.1425-1429
Main Author: Schröder, Kristin
Other Authors: Join, Benoît , Amali, Arlin Jose , Junge, Kathrin , Ribas, Xavi , Costas, Miquel , Beller, Matthias
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201004623
Link: http://search.proquest.com/docview/849429489/?pq-origsite=primo
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title: A biomimetic iron catalyst for the epoxidation of olefins with molecular oxygen at room temperature.
format: Article
creator:
  • Schröder, Kristin
  • Join, Benoît
  • Amali, Arlin Jose
  • Junge, Kathrin
  • Ribas, Xavi
  • Costas, Miquel
  • Beller, Matthias
subjects:
  • Alkenes–Chemistry
  • Biomimetic Materials–Chemistry
  • Catalysis–Chemistry
  • Imidazoles–Chemistry
  • Iron–Chemistry
  • Oxidation-Reduction–Chemistry
  • Oxygen–Chemistry
  • Stilbenes–Chemistry
  • Temperature–Chemistry
  • Alkenes
  • Imidazoles
  • Stilbenes
  • Imidazole
  • Iron
  • Oxygen
ispartof: Angewandte Chemie (International ed. in English), February 7, 2011, Vol.50(6), pp.1425-1429
description: It's no sacrifice: A bio‐inspired iron system, in which a β‐keto ester serves as a sacrificial cosubstrate, readily epoxidizes olefins under ambient conditions with air. Aromatic olefins are oxidized in high yields with excellent chemoselectivity. Mechanistic investigations point out substantial differences to well‐known radical‐based autoxidations.
language: eng
source:
identifier: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201004623
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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titleA biomimetic iron catalyst for the epoxidation of olefins with molecular oxygen at room temperature.
creatorSchröder, Kristin ; Join, Benoît ; Amali, Arlin Jose ; Junge, Kathrin ; Ribas, Xavi ; Costas, Miquel ; Beller, Matthias
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identifierE-ISSN: 1521-3773 ; DOI: 10.1002/anie.201004623
subjectAlkenes–Chemistry ; Biomimetic Materials–Chemistry ; Catalysis–Chemistry ; Imidazoles–Chemistry ; Iron–Chemistry ; Oxidation-Reduction–Chemistry ; Oxygen–Chemistry ; Stilbenes–Chemistry ; Temperature–Chemistry ; Alkenes ; Imidazoles ; Stilbenes ; Imidazole ; Iron ; Oxygen
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descriptionIt's no sacrifice: A bio‐inspired iron system, in which a β‐keto ester serves as a sacrificial cosubstrate, readily epoxidizes olefins under ambient conditions with air. Aromatic olefins are oxidized in high yields with excellent chemoselectivity. Mechanistic investigations point out substantial differences to well‐known radical‐based autoxidations.
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titleA biomimetic iron catalyst for the epoxidation of olefins with molecular oxygen at room temperature.
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