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On the macrocyclization of the erythromycin core: preorganization is not required.

Free of bias : Preorganization is not a requirement for the efficient cyclization of the erythromycin core, as has always been assumed. This finding has enabled CH oxidative cyclization or Yamaguchi macrocyclization to form stereochemically modified erythromycin structures that were previously inac... Full description

Journal Title: Angewandte Chemie (International ed. in English) February 25, 2011, Vol.50(9), pp.2094-2097
Main Author: Stang, Erik M
Other Authors: White, M Christina
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; DOI: 1521-3773 ; DOI: 10.1002/anie.201007309
Link: http://search.proquest.com/docview/853677041/?pq-origsite=primo
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recordid: proquest853677041
title: On the macrocyclization of the erythromycin core: preorganization is not required.
format: Article
creator:
  • Stang, Erik M
  • White, M Christina
subjects:
  • Cyclization–Chemical Synthesis
  • Erythromycin–Chemistry
  • Lactones–Chemistry
  • Oxidation-Reduction–Chemistry
  • Stereoisomerism–Chemistry
  • Lactones
  • Erythromycin
ispartof: Angewandte Chemie (International ed. in English), February 25, 2011, Vol.50(9), pp.2094-2097
description: Free of bias : Preorganization is not a requirement for the efficient cyclization of the erythromycin core, as has always been assumed. This finding has enabled CH oxidative cyclization or Yamaguchi macrocyclization to form stereochemically modified erythromycin structures that were previously inaccessible by using the traditional biasing element approach (see scheme; PG=protecting group).
language: eng
source:
identifier: E-ISSN: 1521-3773 ; DOI: 1521-3773 ; DOI: 10.1002/anie.201007309
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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descriptionFree of bias : Preorganization is not a requirement for the efficient cyclization of the erythromycin core, as has always been assumed. This finding has enabled CH oxidative cyclization or Yamaguchi macrocyclization to form stereochemically modified erythromycin structures that were previously inaccessible by using the traditional biasing element approach (see scheme; PG=protecting group).
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