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The complete characterization of a reduced biomimetic [2Fe-2S] cluster.

: A biomimetic [2 Fe‐2 S] cluster is characterized crystallographically in both the [FeFe] and the mixed‐valent [FeFe] forms—the [2 Fe‐2 S] cores show only minor geometric differences. The reduced form has an =1/2 ground state and the unpaired electron is partially delocalized over the cluster core.... Full description

Journal Title: Angewandte Chemie (International ed. in English) September 19, 2011, Vol.50(39), pp.9191-9194
Main Author: Albers, Antonia
Other Authors: Demeshko, Serhiy , Dechert, Sebastian , Bill, Eckhard , Bothe, Eberhard , Meyer, Franc
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; DOI: 1521-3773 ; DOI: 10.1002/anie.201100727
Link: http://search.proquest.com/docview/890679566/?pq-origsite=primo
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title: The complete characterization of a reduced biomimetic [2Fe-2S] cluster.
format: Article
creator:
  • Albers, Antonia
  • Demeshko, Serhiy
  • Dechert, Sebastian
  • Bill, Eckhard
  • Bothe, Eberhard
  • Meyer, Franc
subjects:
  • Biomimetic Materials–Chemistry
  • Crystallography, X-Ray–Chemistry
  • Ferredoxins–Chemistry
  • Iron–Chemistry
  • Molecular Conformation–Chemistry
  • Oxidation-Reduction–Chemistry
  • Sulfur–Chemistry
  • Ferredoxins
  • Sulfur
  • Iron
ispartof: Angewandte Chemie (International ed. in English), September 19, 2011, Vol.50(39), pp.9191-9194
description: : A biomimetic [2 Fe‐2 S] cluster is characterized crystallographically in both the [FeFe] and the mixed‐valent [FeFe] forms—the [2 Fe‐2 S] cores show only minor geometric differences. The reduced form has an =1/2 ground state and the unpaired electron is partially delocalized over the cluster core. The experimental effective coupling constant predicts the position of the intervalence charge transfer band in the IR regime.
language: eng
source:
identifier: E-ISSN: 1521-3773 ; DOI: 1521-3773 ; DOI: 10.1002/anie.201100727
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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titleThe complete characterization of a reduced biomimetic [2Fe-2S] cluster.
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description: A biomimetic [2 Fe‐2 S] cluster is characterized crystallographically in both the [FeFe] and the mixed‐valent [FeFe] forms—the [2 Fe‐2 S] cores show only minor geometric differences. The reduced form has an =1/2 ground state and the unpaired electron is partially delocalized over the cluster core. The experimental effective coupling constant predicts the position of the intervalence charge transfer band in the IR regime.
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