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[RhIIICp*]-catalyzed dehydrogenative aryl-aryl bond formation.

Directed, undirected! Rhodium(III)‐catalyzed double CH bond activation (one directed, one undirected) provides an efficient route to biaryls (see scheme; DG=directing group). Significant kinetic isotope effects for both reaction partners and H/D scrambling between them are interesting experimental f... Full description

Journal Title: Angewandte Chemie (International ed. in English) February 27, 2012, Vol.51(9), pp.2247-2251
Main Author: Wencel-Delord, Joanna
Other Authors: Nimphius, Corinna , Patureau, Frederic W , Glorius, Frank
Format: Electronic Article Electronic Article
Language: English
Subjects:
ID: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201107842
Link: http://search.proquest.com/docview/923575184/?pq-origsite=primo
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recordid: proquest923575184
title: [RhIIICp*]-catalyzed dehydrogenative aryl-aryl bond formation.
format: Article
creator:
  • Wencel-Delord, Joanna
  • Nimphius, Corinna
  • Patureau, Frederic W
  • Glorius, Frank
subjects:
  • Benzamides–Chemistry
  • Catalysis–Chemistry
  • Hydrocarbons, Aromatic–Chemistry
  • Rhodium–Chemistry
  • Stereoisomerism–Chemistry
  • Benzamides
  • Hydrocarbons, Aromatic
  • Rhodium
ispartof: Angewandte Chemie (International ed. in English), February 27, 2012, Vol.51(9), pp.2247-2251
description: Directed, undirected! Rhodium(III)‐catalyzed double CH bond activation (one directed, one undirected) provides an efficient route to biaryls (see scheme; DG=directing group). Significant kinetic isotope effects for both reaction partners and H/D scrambling between them are interesting experimental findings. While the mechanism is still unclear, a rhodium(V) species is invoked in the catalytic cycle.
language: eng
source:
identifier: E-ISSN: 1521-3773 ; DOI: 10.1002/anie.201107842
fulltext: fulltext
issn:
  • 15213773
  • 1521-3773
url: Link


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identifierE-ISSN: 1521-3773 ; DOI: 10.1002/anie.201107842
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descriptionDirected, undirected! Rhodium(III)‐catalyzed double CH bond activation (one directed, one undirected) provides an efficient route to biaryls (see scheme; DG=directing group). Significant kinetic isotope effects for both reaction partners and H/D scrambling between them are interesting experimental findings. While the mechanism is still unclear, a rhodium(V) species is invoked in the catalytic cycle.
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